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• W2322445900 endingPage "8767" @default.
• W2322445900 startingPage "8759" @default.
• W2322445900 abstract "Thin films of four-coordinated perfluoroalkyl-substituted phthalocyanines were prepared by physical vapor deposition. The electrochemical redox characteristics and simultaneous changes in the optical absorbance spectra of the films (40−215 nm) in contact with an aqueous LiCl electrolyte for charge compensation were compared to results obtained for the molecules dissolved in an organic solvent. A positive shift of the potential of the first ring-centered reduction relative to the unsubstituted or perfluorinated phthalocyanines was confirmed for solutions and clearly established for thin films. Following a conditioning of the films during the first reduction, chemically reversible and thermodynamically quasi-reversible reduction and reoxidation reactions were observed. A clear correlation of the injected charge with the appearance of isosbestic points characterized the reaction as a one-electron reduction. Diffusion limitation by charge-balancing lithium counterions could be detected only for thicker films leading to high switching speeds of the electrochromic reaction in thinner films of about a second and thus rendering the materials interesting candidates for organic electrochromic display applications." @default.
• W2322445900 created "2016-06-24" @default.
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• W2322445900 date "2011-04-12" @default.
• W2322445900 modified "2023-09-26" @default.
• W2322445900 title "Electrochromic Switching of Evaporated Thin Films of Bulky, Electronic Deficient Metallo-Phthalocyanines" @default.
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• W2322445900 doi "https://doi.org/10.1021/jp2010748" @default.
• W2322445900 hasPublicationYear "2011" @default.
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