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- W2322458045 abstract "Germanium combined with high-κ dielectrics is investigated for the next generations of CMOS devices. Therefore, we study reaction mechanisms for Al2O3 atomic layer deposition on sulfur passivated Ge using calculations based on density functional theory and total reflection X-ray fluorescence (TXRF). TXRF indicates 6 S/nm2 and 4 Al/nm2 after the first TMA/H2O reaction cycle, and growth inhibition from the second reaction cycle on. Calculations are performed on molecular clusters representing −GeSH surface sites. The calculations confirm that the TMA reaction does not affect the S content. On fully SH-terminated Ge, TMA favorably reacts with up to three −GeSH sites, resulting in a near tetrahedral Al coordination. Electron deficient structures with a Ge–S site shared between two Al atoms are proposed. The impact of the cluster size on the structures and reaction energetics is systematically investigated." @default.
- W2322458045 created "2016-06-24" @default.
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- W2322458045 date "2011-08-15" @default.
- W2322458045 modified "2023-09-30" @default.
- W2322458045 title "Mechanisms for the Trimethylaluminum Reaction in Aluminum Oxide Atomic Layer Deposition on Sulfur Passivated Germanium" @default.
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- W2322458045 doi "https://doi.org/10.1021/jp206070y" @default.
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