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- W2322671741 abstract "We demonstrate that photon antibunching observed for individual nanocrystal quantum dots (NQDs) can be transformed into photon bunching characterized by super-Poissonian statistics when they are coupled to metal nanostructures (MNs). This observation indicates that, while the quantum yield of a biexciton (${Q}_{2mathrm{X}}$) is lower than that of a single exciton (${Q}_{1mathrm{X}}$) in freestanding NQDs, ${Q}_{2mathrm{X}}$ becomes greater than ${Q}_{1mathrm{X}}$ in NQDs coupled to MNs. This unique phenomenon is attributed to metal-induced quenching with a rate that scales more slowly with exciton multiplicity than the radiative decay rate and dominates over other nonradiative decay channels for both single excitons and biexcitons." @default.
- W2322671741 created "2016-06-24" @default.
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- W2322671741 date "2013-03-11" @default.
- W2322671741 modified "2023-10-09" @default.
- W2322671741 title "Super-Poissonian Statistics of Photon Emission from Single CdSe-CdS Core-Shell Nanocrystals Coupled to Metal Nanostructures" @default.
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- W2322671741 doi "https://doi.org/10.1103/physrevlett.110.117401" @default.
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