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• W2322762246 endingPage "3151" @default.
• W2322762246 startingPage "3147" @default.
• W2322762246 abstract "Abstract CO 2 capture has attracted increasing attention owing to its contribution to global warming and climate change as a greenhouse gas. As an alternative strategy to transition‐metal‐based chemistry and catalysis, frustrated Lewis pairs have been developed to sequester CO 2 efficiently under mild conditions. However, the mechanism of CO 2 sequestration with amidophosphoranes remains unclear. Herein, we present a thorough density functional theory study on a series of amidophosphoranes. Our results reveal that the interplay of the ring strain and the trans influence determines the reactivities, thus opening a new avenue to the design of frustrated Lewis pairs for CO 2 capture." @default.
• W2322762246 created "2016-06-24" @default.
• W2322762246 creator A5012980782 @default.
• W2322762246 creator A5047487011 @default.
• W2322762246 date "2013-09-03" @default.
• W2322762246 modified "2023-10-18" @default.
• W2322762246 title "Mechanistic Insight into the CO₂Capture by Amidophosphoranes: Interplay of the Ring Strain and the<i>trans</i>Influence Determines the Reactivity of the Frustrated Lewis Pairs" @default.
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• W2322762246 doi "https://doi.org/10.1002/asia.201300864" @default.
• W2322762246 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/24038966" @default.
• W2322762246 hasPublicationYear "2013" @default.
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