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- W2322796872 abstract "We report the results of an X-ray photoelectron spectroscopic (XPS) investigation of the total valence-band density of states (VBDOS) of Tl 3 AsSe 3 , a ternary sulfosalt-type crystal. The XPS-VBDOS consists of three regions. The upper portion of the VBDOS, Region I, is approximately 8 eV wide and exhibits three distinct broad features (at ∼1.7, ∼4, and ∼6.5 eV below the valence-band maximum). This region is derived mostly from Se 4p orbitals with some contribution from Tl 6s orbitals. Region II lies to the low binding-energy side of and is partially obscured by the Tl 5 d core level. These bands of mostly As 4s origin are broad and centered approximately at 10 eV. The last region (III) consists of the very intense Tl 5 d 3/2 and Tl 5 d 5/2 core levels at 14.8 and 12.6 eV below the top of the valence-band maximum, respectively. These levels probably obscure the much weaker, lowermost, nearly core-like Se 4s derived bands. These results are in qualitatively good agreement with our recent LCAO calculations with the most serious deviation being the position of the lowermost band." @default.
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- W2322796872 date "1980-01-01" @default.
- W2322796872 modified "2023-10-17" @default.
- W2322796872 title "XPS Valence-Band Densities of States of Ternary Chalcogenide Crystals: Application to Tl<sub>3</sub>AsSe<sub>3</sub>" @default.
- W2322796872 doi "https://doi.org/10.7567/jjaps.19s3.377" @default.
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