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- W2323051273 abstract "The effect of the quadrupole moment induced in the $1s$ shell on the nuclear quadrupole coupling $q$ in the ${mathrm{Li}}_{2}$ molecule has been investigated for several wave functions. For the most accurate variational wave function of James, the inclusion of the induced moment gives $frac{q}{2e}=ensuremath{-}0.00106{{a}_{mathrm{H}}}^{ensuremath{-}3}$. This result, together with the quadrupole coupling $eqQ=+0.060$ Mc/sec for ${mathrm{Li}}^{7}$, leads to a negative value of the quadrupole moment $Q({mathrm{Li}}^{7})$. However the value of $q$ is so close to zero that the magnitude and even the sign of $Q$ is uncertain. The value of $frac{1}{q}$ which determines $Q$ is very sensitive to changes in the molecular wave function, and it is shown that a small modification of the James wave function would lead to a negative $Q({mathrm{Li}}^{7})$ which agrees in order of magnitude with the prediction of the nuclear shell model. Calculations of $q$ were also carried out for the Heitler-London and Coulson-Duncanson wave functions for the ${mathrm{Li}}_{2}$ molecule." @default.
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- W2323051273 date "1953-12-15" @default.
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- W2323051273 title "Nuclear Quadrupole Coupling in the<mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML display=inline><mml:mrow><mml:msub><mml:mrow><mml:mi mathvariant=normal>Li</mml:mi></mml:mrow><mml:mrow><mml:mn>2</mml:mn></mml:mrow></mml:msub></mml:mrow></mml:math>Molecule" @default.
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- W2323051273 doi "https://doi.org/10.1103/physrev.92.1460" @default.
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