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- W2323296597 endingPage "1035" @default.
- W2323296597 startingPage "981" @default.
- W2323296597 abstract "The present report intends to highlight the main lines of our investigation on a series of modular domino reactions focusing on a multi-task reagent, namely Pb(OAc)4 in conjunction with an olefin as a source of complexity. It covers the design, development, and mechanistic aspects of a domino methodology discovered in our laboratory, which presents numerous challenges, including issues of chemo-, regio-, and diastereoselectivities. The principal characteristic of the chemistry presented is the potential of creating cyclic arrays that can be suitably functionalized for subsequent conversion into various complex systems. The effects of systematic variation of domino promoter, substitution pattern, solvent, temperature, and microwave activation on the outcome of the domino reaction are presented. In general terms, the domino chemistry reported here could be conveniently divided into two categories, dealing with first and second generation domino probes based on the nature of the angular substituent, each of which will be addressed in turn. This review is not intended to give an extensive coverage of the various uses of Pb(OAc)4 in synthesis reported in the literature, but will expose relevant reactions where appropriate focusing exclusively on multi-stage transformations initiated by the reagent." @default.
- W2323296597 created "2016-06-24" @default.
- W2323296597 creator A5028088287 @default.
- W2323296597 creator A5048208755 @default.
- W2323296597 creator A5048426778 @default.
- W2323296597 creator A5073073439 @default.
- W2323296597 creator A5090193661 @default.
- W2323296597 date "2015-10-01" @default.
- W2323296597 modified "2023-10-16" @default.
- W2323296597 title "Stimulating excursions into organolead chemistry: modular domino sequences triggered by oxidative cleavage" @default.
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