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• W2323766904 abstract "We exploit the relationship between high harmonic generation (HHG) and the molecular photorecombination dipole to extract the molecular-frame differential photoionization cross section (PICS) in the extreme ultraviolet (XUV) for molecular nitrogen. A shape resonance and a Cooper-type minimum are reflected in the pump-probe time delay measurements of different harmonic orders, where high-order rotational revivals are observed in N${}_{2}$. We observe the energy- and angle-dependent Cooper minimum and shape resonance directly in the laboratory-frame HHG yield by achieving a high degree of alignment, $ensuremath{langle}{mathrm{cos}}^{2}ensuremath{theta}ensuremath{rangle}ensuremath{ge}0.8$. The interplay between PICS and rotational revivals is confirmed by simulations using the quantitative rescattering theory. Our method of extracting molecular-frame structural information points the way to similar measurements in more complex molecules." @default.
• W2323766904 created "2016-06-24" @default.
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• W2323766904 date "2013-10-17" @default.
• W2323766904 modified "2023-09-27" @default.
• W2323766904 title "Measuring the angle-dependent photoionization cross section of nitrogen using high-harmonic generation" @default.
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• W2323766904 doi "https://doi.org/10.1103/physreva.88.043421" @default.
• W2323766904 hasPublicationYear "2013" @default.
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