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• W2323923022 startingPage "1416" @default.
• W2323923022 abstract "Rhodium(I) silylamide complexes supported by the 1,2-bis(di-tert-butylphosphino)ethane (dtbpe) ligand have been prepared and their structures and reactivity studied. Although the complexes degrade over time to release the corresponding silylamines, they react cleanly with silver(I) salts to transfer the amido group at ambient temperature. The bis(trimethylsilyl)amide complex (dtbpe)Rh–N(TMS)2 reacts with CO2 to form a carbamate complex that decomposes via loss of hexamethyldisiloxane to form a bis(μ-isocyanate) dimer, suggesting that silylamides may be useful nitrene-group and nitrogen-atom sources through selective N–Si bond cleavage." @default.
• W2323923022 created "2016-06-24" @default.
• W2323923022 creator A5018110037 @default.
• W2323923022 creator A5038379932 @default.
• W2323923022 creator A5088283556 @default.
• W2323923022 date "2014-03-07" @default.
• W2323923022 modified "2023-10-16" @default.
• W2323923022 title "Synthesis and Reactivity of Three-Coordinate (dtbpe)Rh Silylamides: CO₂ Bond Cleavage by a Rhodium(I) Disilylamide" @default.
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• W2323923022 doi "https://doi.org/10.1021/om401130q" @default.
• W2323923022 hasPublicationYear "2014" @default.
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