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- W2324166434 abstract "Lithium organics with a C5 perimeter are the most prominent class of compounds in s-block metal organic chemistry to introduce bulky haptotropic bound substituents in organometallic complexes. In this paper we present some coordination patterns. (η5-Cp)Li(PMDETA) (1), (η5-Cp)Li(TMEDA) (2), and (η5-Cp)Li(DME) (3) reveal the electron-releasing capacity of the donor base: The better the density supply from the base, the longer the Li···Cpcenter distance. The donor base DIGLYME gives the solvent-separated ion pair (SSIP) [(DIGLYME)2Li][(η5-Cp)2Li] (4). The contact ion pair (η2-Ind)Li(PMDETA) (5) shows an unprecedented strong C–H···π interaction of a PMDETA methyl group to the center of the C6 perimeter of an indenyl anion. {(η5-Ind)Li(μ-DME)Li(η5-Ind)} (6) is a unique DME-bridged dimer, while [(DIGLYME)2Li][Ind] (7) crystallizes as a SSIP." @default.
- W2324166434 created "2016-06-24" @default.
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- W2324166434 date "2011-08-01" @default.
- W2324166434 modified "2023-10-03" @default.
- W2324166434 title "Revealing Coordination Patterns in C<sub>5</sub>-Cyclic Lithium Organics" @default.
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- W2324166434 doi "https://doi.org/10.1021/om200471e" @default.
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