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• W2324166616 abstract "From electric conductivity measurements of uranyl nitrate hexahydrate solutions in solvents of dielectric constants ranging from 7 to 109 (TBP, methylisobutylketone, methylethylketone, acetone, acetylacetone, ethanol, methanol, acetonitrile, water and formamide) the dissociation constants were calculated for this salt. These constants are of the order of 10−11 (in TBP) to 10−1 triplet-ions UO2(NO3)3- with dissociation constants of the order 10−8 to 10−2. Bjerrum's parameters (in formamide). It has been found that within a certain concentration range the uranyl nitrate forms a were calculated as well. Their very low values pointed to the presence of covalent binding between uranyl and nitrate. Therefore the values of the a parameter only allow one to draw qualitative conclusions. By using Gilkerson's derivation of the dissociation constant, the solvation of uranyl nitrate in organic solvents was examined. In several solvents the energy of solvation has the same value and the water and solvent molecules compete in the primary solvation shell. In strongly polar solvents the water molecules in the solvation shell are completely substituted by solvent molecules forming a stable complex species. The parameter a was now calculated on the basis of Gilkerson's relation for several solvents giving a constant value 2·1 Å." @default.
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• W2324166616 date "1961-11-01" @default.
• W2324166616 modified "2023-10-18" @default.
• W2324166616 title "The behaviour and structure of uranyl nitrate in organic solvents—I" @default.
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• W2324166616 doi "https://doi.org/10.1016/0022-1902(61)80467-3" @default.
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