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- W2324330239 abstract "Nanosecond time-resolved electron paramagnetic resonance (TREPR) spectroscopy has been utilized at T = 77 K to characterize alkyl side-chain effects on geometries and on the electronic couplings (VCR) of transient charge-separated (CS) states in the photoactive layers fabricated by the spin-coating of mixed solutions of regioregular polyalkylthiophenes (RR-P3AT) and [6,6]-C61-butyric acid methyl ester (PCBM). By increasing the alkyl side-chain number from 6 to 12 in P3AT, a highly distant and long-lived CS state has been obtained. This result is explained by a coupling of the hole dissociation to the polymer librations by the side-chains. From an exponential decay of VCR with respect to the CS distance, the attenuation factor (βe) has been determined to be βe = 0.2 Å(-1). Such a long-range tunneling feature is explained by the generations of the shallowly trapped, delocalized electron-hole pairs by the dissociation of the hole toward π-stacking directions at the organic photovoltaic interface." @default.
- W2324330239 created "2016-06-24" @default.
- W2324330239 creator A5016653529 @default.
- W2324330239 creator A5026498329 @default.
- W2324330239 creator A5037644583 @default.
- W2324330239 date "2013-12-24" @default.
- W2324330239 modified "2023-09-27" @default.
- W2324330239 title "Time-Resolved EPR Study of Electron–Hole Dissociations Influenced by Alkyl Side Chains at the Photovoltaic Polyalkylthiophene:PCBM Interface" @default.
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- W2324330239 doi "https://doi.org/10.1021/jz402300m" @default.
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