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- W2324582303 endingPage "5221" @default.
- W2324582303 startingPage "5218" @default.
- W2324582303 abstract "Comprehensive utilization of both electronic and steric properties of ligands in homogeneous gold catalysis is achieved in the regiodivergent intramolecular hydroarylation of alkynes. A flexible electron-deficient phosphite ligand, combined with the readily transformable directing group methoxyl amide, is attached to a cationic Au(I) center in three-coordinate mode, affording sterically hindered ortho-position cyclization. Meanwhile, para-position cyclization is exclusively achieved with the assistance of a rigid electron-abundant phosphine ligand-based Au(I) catalyst, in which ligands manifest the compensating effect for cyclization through steric hindrance and electronic properties. By combining gold with silver catalysts, tetrahydropyrroloquinolinones possessing a congested tricyclic structure are obtained via a proven Au/Ag relay catalytic process." @default.
- W2324582303 created "2016-06-24" @default.
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- W2324582303 date "2016-04-18" @default.
- W2324582303 modified "2023-10-16" @default.
- W2324582303 title "Utility of Ligand Effect in Homogenous Gold Catalysis: Enabling Regiodivergent π-Bond-Activated Cyclization" @default.
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- W2324582303 doi "https://doi.org/10.1021/jacs.6b01707" @default.
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