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• W2325579897 abstract "The reaction of O(2) with an adlayer of the oligopyridine 2-phenyl-4,6-bis(6-(pyridine-2-yl)-4-(pyridine-4-yl)-pyridine-2-yl)pyrimidine (2,4'-BTP), adsorbed on the (111) surfaces of silver and gold and on HOPG--which can be considered as a model system for inorganic|organic contacts--was investigated by fast scanning tunneling microscopy (video STM) and dispersion corrected density functional theory (DFT-D) calculations. Only on Ag(111), oxidation of the 2,4'-BTP adlayer was observed, which is related to the fact that under the experimental conditions O(2) adsorbs dissociatively on this surface leading to reactive O adatoms, but not on Au(111) or HOPG . There is a distinct regiospecifity of the oxidation reaction caused by intermolecular interactions. In addition, the oxidation leads to a chiral ordering. The relevance of these findings for reactions involving organic monolayers is discussed." @default.
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• W2325579897 date "2012-05-17" @default.
• W2325579897 modified "2023-10-10" @default.
• W2325579897 title "Oxidation of an Organic Adlayer: A Bird’s Eye View" @default.
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• W2325579897 doi "https://doi.org/10.1021/ja302593v" @default.
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