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• W2326172743 abstract "A new family of microporous polymeric organic frameworks (POF)s is described. The POFs are assembled from phlorglucinol (1,3,5-trihydroxybenzene) and several benzaldehyde derivatives under solvothermal conditions using Bakelite type chemistry of forming C−C bonds without any catalyst. The materials exhibit semiconductor-like optical absorption properties with energy gaps in the range of 1.5−2.5 eV. The new materials form as uniform, microporous, spherical particles and exhibit surface areas up to 917 m2 g−1. The micropores have a very uniform size as the gas adsorption isotherms of these amorphous materials are similar to those of crystalline microporous zeolites. The micropores are internally decorated with a large number of −OH reactive groups which are available for functionalization. The POFs capture as much as 18% of their mass of CO2 at atmospheric pressure which is significantly larger than other porous polymers including systems which exhibit much larger surface areas; sodium-functionalized POFs exhibit enhanced heat of adsorption for H2 of 9 kJ/mol compared to pristine POF at 8.3 kJ/mol." @default.
• W2326172743 created "2016-06-24" @default.
• W2326172743 creator A5035758112 @default.
• W2326172743 creator A5090274462 @default.
• W2326172743 date "2011-03-16" @default.
• W2326172743 modified "2023-10-18" @default.
• W2326172743 title "Phloroglucinol Based Microporous Polymeric Organic Frameworks with −OH Functional Groups and High CO₂ Capture Capacity" @default.
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• W2326172743 doi "https://doi.org/10.1021/cm103206x" @default.
• W2326172743 hasPublicationYear "2011" @default.
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