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- W2326481964 abstract "In this work, we synthesized gold clusters, Aun (n = 10, 18, 25, 39), with atomically controlled sizes on hydroxyapatite (HAP) and studied the catalysis for aerobic oxidation of cyclohexane. These Aun/HAP catalysts could efficiently oxidize cyclohexane to cyclohexanol and cyclohexanone. The turnover frequency monotonically increased with an increase in the size, reaching values as high as 18 500 h−1 Au atom−1 at n = 39, and thereafter decreased with a further increase in n up to n ∼ 85. This finding provides a fundamental insight into size-specific catalysis of gold in the cluster regime (diameter < 2 nm) and a guiding principle for rational design of Au cluster-based catalysts." @default.
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- W2326481964 date "2010-12-10" @default.
- W2326481964 modified "2023-10-09" @default.
- W2326481964 title "Aerobic Oxidation of Cyclohexane Catalyzed by Size-Controlled Au Clusters on Hydroxyapatite: Size Effect in the Sub-2 nm Regime" @default.
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- W2326481964 doi "https://doi.org/10.1021/cs100043j" @default.
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