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- W2326521714 abstract "To investigate the correlation between the activation energy E ac and electronic structure near the band gap for impurity-type H + -ion conductors, we measured infrared reflectivity spectra of sintered BaCe 1- x M x O 3 ( x =0, 0.10, 0.15 for M = Nd and x =0.05, 0.1 for M = Gd) at room temperature, and estimated optical dielectric constant ε ∞ and the phonon frequencies of LO- and TO-modes with Kramers–Kronig analysis. We found a clear proportionality represented as E ac - 0.14=[1/( ε ∞ -1.4)]. The proportional form is shifted from that of superionic conductor. For the origin of the shift, we attribute weakened influence of the Coulomb force of the host lattice on mobile H + -ion. This mechanism is confirmed from the volume and mass dependences of E ac values, and also from reasonable interpretation about smaller E ac value of AB 1- x M x O 3 than that of ABO 3 with respect to the impurity electronic levels near the band edge." @default.
- W2326521714 created "2016-06-24" @default.
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- W2326521714 date "2010-01-01" @default.
- W2326521714 modified "2023-09-27" @default.
- W2326521714 title "Relationship Between Optical Dielectric Constant and Ionic Activation Energy in Perovskite-Type Proton Conductors BaCe<sub>1-<i>x</i></sub>M<sub><i>x</i></sub>O<sub>3</sub>(M = Nd and Gd )" @default.
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- W2326521714 doi "https://doi.org/10.1143/jpsjs.79sa.37" @default.
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