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- W2326879056 abstract "Ni-Based catalysts using mixed oxides of Al2O3–SiO2, Al2O3–TiO2, TiO2–SiO2, and TiO2–ZrO2 as supports were evaluated for hydrotreatments using guaiacol as the model compound and characterized by N2 physical adsorption, X-ray diffraction (XRD), temperature-programmed desorption of ammonia (NH3-TPD), and temperature-programmed reduction of hydrogen (H2-TPR) techniques. The influence of the support, solvent, reaction temperature, and pressure on guaiacol conversion and product distributions were determined. Guaiacol conversion of 100% with cyclohexane selectivity of 86.4% was obtained over the Ni/TiO2–ZrO2 catalyst at the conditions of 300 °C, 4.0 MPa H2 pressure, and decalin solvent. Furthermore, this system is also efficient for real bio-oil, where nearly 19.3% of the upgraded bio-oil yield was achieved under the optimal conditions determined for guaiacol. Gas chromatography–mass spectrometry (GC–MS) analysis showed that the principal components were phenolic compounds, while the content of acids and aldehydes was negligible. The pH of bio-oil increased from 2.38 to 4.21, and the high heating value drastically increased from 13.1 to 25.8 MJ/kg." @default.
- W2326879056 created "2016-06-24" @default.
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- W2326879056 date "2014-04-08" @default.
- W2326879056 modified "2023-10-05" @default.
- W2326879056 title "Catalytic Upgrading of Bio-oil over Ni-Based Catalysts Supported on Mixed Oxides" @default.
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- W2326879056 doi "https://doi.org/10.1021/ef402421j" @default.
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