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• W2326921495 abstract "Abstract In this study, mesoporous graphitic carbon nitride (mpg-C 3 N 4 ) nanosheets with high surface area (317 m 2  g −1 ) were obtained by using SBA-15 as a hard-template, and CdLa 2 S 4 nanoparticles were successfully grown on these mpg-C 3 N 4 nanosheets via a facile hydrothermal method. The as-synthesized CdLa 2 S 4 /mpg-C 3 N 4 hybrids were characterized by X-ray diffraction (XRD), transmission electron microscopy (TEM), high-resolution transmission electron microcopy (HRTEM), energy-dispersive X-ray spectroscopy (EDS), X-ray photoelectron spectroscopy (XPS), N 2 adsorption-desorption, ultraviolet–visible diffuse reflection spectroscopy (DRS). Compared with pure CdLa 2 S 4 , the CdLa 2 S 4 /mpg-C 3 N 4 hybrid materials displayed higher photocatalytic H 2 evolution performance under the visible light (λ > 420 nm) using Na 2 S and Na 2 SO 3 as the sacrificial agent. The optimal content of mpg-C 3 N 4 was about 20 wt% and the corresponding photocatalytic H 2 evolution was 5984.8 μmol h −1  g −1 (with an apparent quantum efficiency of 7.1% at 420 nm), which was 7.7 times higher than that of pure CdLa 2 S 4 . The results of photoluminescence (PL) and photocurrent response demonstrated that the recombination of photo-generated electron-hole pairs was effectively inhibited due to the well-matched band structure and intimate contact interfaces of CdLa 2 S 4 and mpg-C 3 N 4 . Based on the results and analysis, a possible enhanced photocatalytic activity mechanism of CdLa 2 S 4 /mpg-C 3 N 4 composites was also proposed." @default.
• W2326921495 created "2016-06-24" @default.
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• W2326921495 date "2016-09-01" @default.
• W2326921495 modified "2023-09-28" @default.
• W2326921495 title "Highly efficient photocatalytic H2 evolution from water over CdLa2S4/mesoporous g-C3N4 hybrids under visible light irradiation" @default.
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• W2326921495 doi "https://doi.org/10.1016/j.apcatb.2016.03.074" @default.
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