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• W2327094902 abstract "A ruthenium(II) complex derived from the electron-deficient aromatic carboxylic acid 3-(F3C)C6H4CO2H proved to be a highly efficient catalyst for dehydrative alkyne annulation by NH-free hydroxamic acids in water. The C–H/N–OH functionalization occurred with excellent positional selectivity as well as ample substrate scope, setting the stage for effective intermolecular alkenylations of hydroxamic acids. Detailed mechanistic studies were suggestive of a kinetically relevant C–H metalation by carboxylate assistance along with subsequent migratory alkyne insertion, reductive elimination, and intramolecular oxidative addition." @default.
• W2327094902 created "2016-06-24" @default.
• W2327094902 creator A5008244937 @default.
• W2327094902 creator A5053550707 @default.
• W2327094902 date "2014-10-30" @default.
• W2327094902 modified "2023-10-07" @default.
• W2327094902 title "Dehydrative C–H/N–OH Functionalizations in H₂O by Ruthenium(II) Catalysis: Subtle Effect of Carboxylate Ligands and Mechanistic Insight" @default.
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• W2327094902 doi "https://doi.org/10.1021/jo501884v" @default.
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