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• W2327494688 abstract "A comprehensive study of size-dependent initial- and final-state effects in $2p$ x-ray absorption of free, homonuclear $3d$ transition metal clusters from titanium through nickel in a size range of 1--200 atoms is presented. From atom to bulk the $2pensuremath{rightarrow}3d$ excitation in $3d$ transition metals shifts to higher photon energy, which can be explained by increasing valence electron delocalization in the initial state. A cluster-size-dependent decrease of the ${L}_{2,3}$ branching ratio at a constant $2p$ spin-orbit splitting can be attributed to core-hole screening effects for all investigated $3d$ transition metal clusters. For small manganese cluster ions, highly localized $3d$ orbitals with ferromagnetic spin coupling and a filled $3d$ majority spin subband are suggested by the experimental $2p$ x-ray absorption spectra." @default.
• W2327494688 created "2016-06-24" @default.
• W2327494688 creator A5005668022 @default.
• W2327494688 creator A5007837343 @default.
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• W2327494688 creator A5078930430 @default.
• W2327494688 creator A5089135457 @default.
• W2327494688 date "2012-10-01" @default.
• W2327494688 modified "2023-10-01" @default.
• W2327494688 title "Initial- and final-state effects on screening and branching ratio in<mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML display=inline><mml:mrow><mml:mn>2</mml:mn><mml:mi>p</mml:mi></mml:mrow></mml:math>x-ray absorption of size-selected free<mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML display=inline><mml:mrow><mml:mn>3</mml:mn><mml:mi>d</mml:mi></mml:mrow></mml:math>transition metal clusters" @default.
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• W2327494688 doi "https://doi.org/10.1103/physrevb.86.165402" @default.
• W2327494688 hasPublicationYear "2012" @default.
• W2327494688 type Work @default.
• W2327494688 sameAs 2327494688 @default.

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