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• W2327755583 abstract "Nondestructive methods that allow researchers to gather high-resolution quantitative information on a material’s physical properties from inside a working device are increasingly in demand from the scientific community. Synchrotron-based microcomputed X-ray tomography, which enables the fast, full-field interrogation of materials in functional, real-world environments, was used to observe the physical changes of next-generation lithium-ion battery anode materials and architectures. High capacity, nongraphitic anodes were chosen for study because they represent the future direction of the field and one of their recognized limitations is their large volume expansion and contraction upon cycling, which is responsible for their generally poor electrochemical performance. In this work, Cu6Sn5 coated on a three-dimensional copper foam was used to model a high power electrode while laminated silicon particles were used to model a high energy electrode. The electrodes were illuminated in situ and ex situ, respectively, at Sector 2-BM of the Advanced Photon Source. The changes in electrode porosity and surface area were measured and show large differences based on the electrode architecture. This work is one of the first reports of full-field synchrotron tomography on high-capacity battery materials under operating conditions." @default.
• W2327755583 created "2016-06-24" @default.
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• W2327755583 date "2014-03-17" @default.
• W2327755583 modified "2023-09-25" @default.
• W2327755583 title "Full-Field Synchrotron Tomography of Nongraphitic Foam and Laminate Anodes for Lithium-Ion Batteries" @default.
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• W2327755583 doi "https://doi.org/10.1021/am5003124" @default.
• W2327755583 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/24588840" @default.
• W2327755583 hasPublicationYear "2014" @default.
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