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- W2327756051 abstract "‘Slipped’ π−π stacking between flexible macrocycle 14+ (cyclo[2](2,6-di(1H-imidazol-1-yl)pyridine)[2](1,4-dimethylene benzene)) and neutral small molecules induce one-dimensional (1D) ‘sandwich’ chain self-assembly. Unlike most of the reported π−π stacking system, the 1D “sandwich” chain expands with the direction parallel to stacking π surfaces on 14+ and that on molecule 2, 3, 4 or 5 (2 = p-xylene, 3 = benzene-1,4-diamine, 4 = 4,4′-bipyridine, 5 = [1,1′-biphenyl]-4,4′-diol). Moreover, the π−π stacking modes of 1D self-assembly are seriously small molecule adduct dependent. Combined with the other weak interactions (e.g. intermolecular hydrogen bonding), the new substrate design and control strategy can expand the 1D ‘sandwich’ chain (e.g. [14+·4]n) into higher order structure (e.g. two-dimensional (2D) network [14+·4·6]n, 6 = hydroquinone) even in large scale (~280 mg). This 2D network structure, which keeps stable under 423 K, shows highly selective gas absorption of CO2 over N2." @default.
- W2327756051 created "2016-06-24" @default.
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- W2327756051 date "2016-03-24" @default.
- W2327756051 modified "2023-09-27" @default.
- W2327756051 title "Substrate-induced adjustment of “slipped” π–π stacking: en route to obtain 1D sandwich chain and higher order self-assembly supramolecular structures in solid state" @default.
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- W2327756051 doi "https://doi.org/10.1080/10610278.2016.1161196" @default.
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