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- W2328822057 abstract "Various nitrogen-based bridging ligands at the sites of a Cu(111) surface, including μ3-imido and μ2-azavinylidene species, have been identified by surface-sensitive spectroscopies and density functional theory (DFT) calculations. The isolated intermediates demonstrate how several metal atoms acting in concert can usher the conversion from a primary azide into a nitrile end-product. The collection of mechanistic details, the N–N2 bond scission, the sequential β-hydrogen eliminations, and the alterations of the NC unsaturation, illustrates rich information about structures and transformations of N-donor ligands." @default.
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- W2328822057 date "2013-09-26" @default.
- W2328822057 modified "2023-10-18" @default.
- W2328822057 title "Capture of Bridging Imido and Azavinylidene Intermediates Engaged in Nitrogen Functionality Changes from Primary Azide to Nitrile on a Copper Surface" @default.
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- W2328822057 doi "https://doi.org/10.1021/jp407434z" @default.
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