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• W2328964038 abstract "We report a combined experimental and theoretical study investigating small zinc oxide clusters. A laser vaporization source and a time-of-flight (TOF) mass spectrometer are employed to produce and identify anionic clusters in the Zn(n)O(m) (n = 1-6, m = 1-7) size regime. The adiabatic detachment energy (ADE) and vertical detachment energy (VDE) of Zn(3)O(3)(-) and Zn(3)O(4)(-) clusters are determined via anion photoelectron spectroscopy. We have utilized density functional theory (DFT) calculations to explore the possible geometries of neutral and anionic Zn(3)O(m) (m = 3-5) clusters, while the theoretical ADE and VDE values are compared with experimental results. The experimentally observed relative abundances among the Zn(3)O(m)(-) (m = 3-5) clusters are investigated through calculations of the detachment energies, dissociation energies, and HOMO-LUMO gaps. We find that the Zn(3)O(3) cluster maintains enhanced stability compared to their oxygen-rich counterparts. Furthermore, by coupling the experimentally obtained photoelectron angular distributions of Zn(3)O(3)(-) and Zn(3)O(4)(-) with electronic structure calculations, the nature of the highest occupied molecular orbitals is discussed, with the goal of aiding the isolation (ligand-capped)/deposition of these building blocks." @default.
• W2328964038 created "2016-06-24" @default.
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• W2328964038 date "2012-12-14" @default.
• W2328964038 modified "2023-10-18" @default.
• W2328964038 title "Investigating the Relative Stabilities and Electronic Properties of Small Zinc Oxide Clusters" @default.
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• W2328964038 doi "https://doi.org/10.1021/jp3029374" @default.
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