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• W2329543859 abstract "The barrier soils used in low-level radioactive waste (LLW) disposal must provide long-term attenuation of radioactive compounds, with a service life in excess of 1000 yr. Although primary to containment theory, knowledge of radionuclide transport via sorption processes is still under development. The current approach to modeling sorption behavior of radioactive compounds to barrier soils relies on experimental data from purified minerals that are not representative of the natural, heterogeneous mineral assemblages found in soils or proposed in practice. In this study, sorption experiments using nonsynthetic barrier soils were conducted to provide a more realistic evaluation of sorption processes involving radioactive compounds. Four liner soils of varying properties were used for experimentation, while uranium acetate dihydrate (UO 2 (C 2 H 3 O 2 ) 2 2 ≤ 2 H 2 O) served as the representative radionuclide. The proportionality of radionuclide sorption to the exchange capacity of soils, as a function of the type and magnitude of the minerals within the soil column, is investigated. Inclusion of carbonate species shows a decrease in sorption capacity, while the presence of amorphous iron increases sorption. Cross-comparisons between sorption behavior of purified clays and iron minerals within the literature to the study soils show a reliance on multiple portions of the mineralogic soil content to account for demonstrated radionuclide sorption capacity." @default.
• W2329543859 created "2016-06-24" @default.
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• W2329543859 date "2014-02-24" @default.
• W2329543859 modified "2023-09-23" @default.
• W2329543859 title "Radionuclide Behavior in Low-Level Radioactive Waste (LLW) Disposal Barrier Materials: Impacts of Sorption" @default.
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• W2329543859 doi "https://doi.org/10.1061/9780784413272.189" @default.
• W2329543859 hasPublicationYear "2014" @default.
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