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- W2329608935 abstract "Hydroxyl radical damage to DNA causes disease, and sulfur and selenium antioxidant coordination to hydroxyl-radical-generating Cu+ is one mechanism for their observed DNA damage prevention. To determine how copper binding results in antioxidant activity, biologically relevant selone and thione ligands and Cu+ complexes of the formula [Tpm*Cu(L)]+ [Tpm* = tris(3,5-dimethylpyrazolyl)methane; L = N,N′-dimethylimidazole selone or thione] were treated with H2O2 and the products analyzed by 1H, 13C{1H}, and 77Se{1H} NMR spectroscopy, mass spectrometry, and X-ray crystallography. Upon H2O2 treatment, selone and thione binding to Cu+ prevents oxidation to Cu2+; instead, the chalcogenone ligand is oxidized. Thus, copper coordination by sulfur and selenium compounds can provide targeted sacrificial antioxidant activity." @default.
- W2329608935 created "2016-06-24" @default.
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- W2329608935 date "2013-10-02" @default.
- W2329608935 modified "2023-10-13" @default.
- W2329608935 title "Oxidation of Biologically Relevant Chalcogenones and Their Cu(I) Complexes: Insight into Selenium and Sulfur Antioxidant Activity" @default.
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- W2329608935 doi "https://doi.org/10.1021/ic401366c" @default.
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