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- W2329941512 endingPage "3730" @default.
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- W2329941512 abstract "Recent developments in stable radical chemistry have afforded heavy atom radicals, neutral open-shell (S = 1/2) molecular species containing heavy p-block elements (S, Se), which display solid-state magnetic properties once considered exclusive to conventional metal-based magnets. These highly spin-delocalized radicals do not associate in the solid state and yet display extensive networks of close intermolecular interactions. Spin density on the heavy atoms allows for increased isotropic and spin-orbit mediated anisotropic exchange effects. Structural variations induced by chemical modification and physical pressure, coupled with ab-initio methods to estimate exchange energies, have facilitated the development of predictive structure/property relationships. These results, coupled with detailed theoretical analyses and magnetic resonance spectroscopic measurements, have provided insight into the magnetic structure of ferromagnetic and spin-canted antiferromagnetic ordered materials as well as an understanding of the importance of spin-orbit coupling contributions to magnetic hysteresis and anisotropy. Isotropic and anisotropic ferromagnetic exchange can also be enhanced indirectly by the incorporation of heavy atoms into nonspin-bearing sites, where they can contribute to multi-orbital spin-orbit coupling." @default.
- W2329941512 created "2016-06-24" @default.
- W2329941512 creator A5052119665 @default.
- W2329941512 creator A5061964321 @default.
- W2329941512 creator A5084118285 @default.
- W2329941512 date "2015-03-13" @default.
- W2329941512 modified "2023-10-16" @default.
- W2329941512 title "Magnetic Ordering and Anisotropy in Heavy Atom Radicals" @default.
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