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• W2330248907 abstract "A series of xMnyCe/hexagonal mesoporous silica (HMS) sorbents with wormhole-like structure was prepared by a sol–gel method, and their performance for hot coal gas desulfurization was investigated at 600 °C. All xMnyCe/HMS sorbents exhibited high breakthrough sulfur capacity, and the utilization of these sorbents was much higher than that of 10Mn/HMS. The breakthrough sulfur capacity over 4Mn1Ce/HMS sorbents was 121.7 mg of S/g of sorbent with the utilization of 82.4%. Such a behavior was maintained in eight consecutive desulfurization–regeneration cycles. The effects of the desulfurization temperature, H2 concentration, and 7% steam on the performance of 4Mn1Ce/HMS were examined. The fresh, used, and regenerated samples were characterized by means of X-ray diffraction, N2 adsorption, Fourier transform infrared absorption spectroscopy, and high-resolution transmission electron microscopy techniques. The results confirmed that the manganese oxide was dispersed highly on the HMS support because of the synergetic effects of manganese oxide and ceria oxide, and the wormhole-like structure in sorbents promoted the diffusion of H2S molecules. The Brunauer–Emmett–Teller results revealed that the wormhole-like mesoporous structure in sorbents remained intact even after the eighth successive desulfurization/regeneration cycle." @default.
• W2330248907 created "2016-06-24" @default.
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• W2330248907 date "2013-11-20" @default.
• W2330248907 modified "2023-10-16" @default.
• W2330248907 title "Fabrication and Performance of <i>x</i>Mn<i>y</i>Ce/Hexagonal Mesoporous Silica Sorbents with Wormhole-Like Framework for Hot Coal Gas Desulfurization" @default.
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• W2330248907 doi "https://doi.org/10.1021/ef4013467" @default.
• W2330248907 hasPublicationYear "2013" @default.
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