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- W2330314463 abstract "Photoluminescence (PL) spectra of natural diamond powders of type IaAB at 300 and 13 K were excited with synchrotron radiation in the wavelength range of 150–260 nm. The spectral features observed in the excitation spectra at 13 K show four vibrational progressions related to nitrogen defects in diamond: A, B, B′, and N3. Progression A has a spacing of 1258 ± 40 cm–1, associated with the N2 (or A) center; progression B has a spacing of 1181 ± 40 cm–1 and progression B′ has a spacing of 744 ± 40 cm–1 related to the N4 (or B) center; and progression N3 has a spacing of 1417 ± 40 cm–1 associated with the N3 center. The PL of these defects comprise continuous emission with two broad lines with maxima of ∼420 and 469 nm at 300 K. Upon excitation with light at wavelengths of <200 nm, the distinct zero-phonon lines of N3 and N4 centers in diamond at a temperature of 13 K become prominent at 416.0 and 491.2 nm, respectively. The vibrational progressions in the photoluminescence excitation (PLE) spectra of N2, N3, and N4 centers in diamond of type IaAB at 13 K are identified for the first time. We suggest the use of PL spectra excited in the region of 160–240 nm to analyze and identify the type of diamond." @default.
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- W2330314463 date "2012-10-19" @default.
- W2330314463 modified "2023-10-09" @default.
- W2330314463 title "Identification of Nitrogen Defects in Diamond with Photoluminescence Excited in the 160–240 nm Region" @default.
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- W2330314463 doi "https://doi.org/10.1021/ac302545u" @default.
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