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- W2330387436 abstract "We report a type of polymer microgel that can undergo a rapid and highly sensitive volume change upon adding H2O2. Such a H2O2-sensitive microgel is made of dextran–tyramine and horseradish peroxidase (HRP), which are interpenetrated in chemically cross-linked gel networks of poly(oligo(ethylene glycol) methacrylates). Unlike the H2O2-sensitive microgels reported in previous arts that typically involve degradation processes related to H2O2-induced cleavability of specific bonds, the proposed microgels can shrink upon adding H2O2 owing to the HRP-catalyzed coupling reaction of tyramine residues via decomposition of H2O2. While a fast (<10 s) and stable shrinkage of the microgels can be reached upon adding H2O2 over a concentration range 50.0 μM–1.0 mM, the response time can be modulated by the dispersion temperature in a nonmonotonous way over 10–38 °C. With the microgels as probes, the H2O2 detection limit was approximately 6.8 μM. In a combined use of the microgels with glucose oxidase for glucose detection, the glucose detection limit was approximately 83.1 μM." @default.
- W2330387436 created "2016-06-24" @default.
- W2330387436 creator A5013563049 @default.
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- W2330387436 date "2014-08-22" @default.
- W2330387436 modified "2023-10-15" @default.
- W2330387436 title "Synthesis and Characterization of Dextran–Tyramine-Based H<sub>2</sub>O<sub>2</sub>-Sensitive Microgels" @default.
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- W2330387436 doi "https://doi.org/10.1021/ma5013368" @default.
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