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- W2330608127 abstract "Uranium and plutonium ions and their complexes play an important role in nuclear fuel reprocessing, and their trace characterization is important in nuclear forensics. In this work, we perform ab initio density functional theory calculations of U and Pu complexes with graphene and graphene oxide to examine the applicability of a graphene-based fissile sensor. We find that graphene needs to be functionalized to act as an effective sensor for detection of fissile materials such as uranium and plutonium complexes. This is because characteristic changes in the plasmonic properties of a finite graphene sheet, molecular electrostatic potentials, and current–voltage characteristics in oxidized graphene nanojunctions are strong signatures of the sorption of uranium or plutonium moieties." @default.
- W2330608127 created "2016-06-24" @default.
- W2330608127 creator A5032050383 @default.
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- W2330608127 date "2013-10-31" @default.
- W2330608127 modified "2023-09-27" @default.
- W2330608127 title "Design of Nanosensors for Fissile Materials in Nuclear Waste Water" @default.
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- W2330608127 doi "https://doi.org/10.1021/jp408247n" @default.
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