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- W2330671038 abstract "The structure of the water/vapor interface covered by a sodium dodecyl sulfate (SDS) monolayer can be remarkably affected by salts in aqueous phase. Molecular dynamics simulations have been performed to reveal the microstructure of the interface with different salts, including NaCl, CaCl2, and MgCl2. The bending modulus κ of the interface exhibits the order: with MgCl2 < with CaCl2 < with NaCl ≈ without salt, while the surface tension γ almost remains unchanged. The smaller κ characterizes larger interfacial fluctuation. In the systems with CaCl2 or MgCl2, the intrinsic density of Na+ adsorbed beside the monolayer is much lower than that without salt or with NaCl due to the adsorption of Ca2+ or Mg2+. However, less Ca2+ or Mg2+ ions enter the hydration shells of sulfate groups while Na+ ions normally coordinate the sulfate groups together with water. So in the systems with CaCl2 or MgCl2, sulfate groups are less bridged by ions and more solvated by water. Thus, the alkyl tails become more disordered. The above microstructure change with the addition of divalent ions leads to more fluctuated interface. This finding helps in understanding the mechanism of the influence of salts on the stability of foam films." @default.
- W2330671038 created "2016-06-24" @default.
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- W2330671038 date "2014-08-13" @default.
- W2330671038 modified "2023-10-16" @default.
- W2330671038 title "Specific Counterion Effects on the Atomistic Structure and Capillary-Waves Fluctuation of the Water/Vapor Interface Covered by Sodium Dodecyl Sulfate" @default.
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- W2330671038 doi "https://doi.org/10.1021/jp505738s" @default.
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