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• W2330822019 endingPage "3325" @default.
• W2330822019 startingPage "3318" @default.
• W2330822019 abstract "Molecular dynamics simulations of anionic sodium decylsulfate and nonionic pentaethylene glycol monodecyl ether micelles in water have been performed to examine the impact of hydrostatic pressure on argon solubilization as a function of pressure. The potential-of-mean force between the micelles and argon demonstrates that nonpolar gases are attracted to the interiors of both micelles. The affinity of argon for micelle interiors, however, decreases with increasing pressure as a result of the comparatively higher molar volume of argon inside assemblies. We evaluate solubility enhancement coefficients, which describe the drop in the solute chemical potential as a function of the micellized surfactant concentration, to quantify the impact of micellization on gas solubilization. While argon is similarly attracted to the hydrophobic cores of both micelles, the gas is more effectively sequestered within nonionic micelles compared with anionic micelles as a result of salting out by charged head groups and accompanying counterions. The solubility enhancement coefficients of both micelles decrease with increasing pressure, reflecting the changing forces observed in the potentials-of-mean force. An analytical liquid drop model is proposed to describe the pressure dependence of argon solubilization within micelles that captures the simulation solubility enhancement coefficients after fitting an effective micelle radius for each surfactant." @default.
• W2330822019 created "2016-06-24" @default.
• W2330822019 creator A5011002849 @default.
• W2330822019 creator A5030112713 @default.
• W2330822019 date "2015-03-10" @default.
• W2330822019 modified "2023-09-26" @default.
• W2330822019 title "Effect of Hydrostatic Pressure on Gas Solubilization in Micelles" @default.
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• W2330822019 doi "https://doi.org/10.1021/la503646z" @default.
• W2330822019 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/25730396" @default.
• W2330822019 hasPublicationYear "2015" @default.
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