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• W2331028144 abstract "The reaction mechanism of the high-temperature water–gas shift (HT-WGS) reaction catalyzed by chromium–iron oxide catalysts for H2 production has been studied for 100 years with two reaction mechanisms proposed: redox and associative (involving surface HCOO*). Direct experimental support for either mechanism, however, is still lacking, which hinders a thorough understanding of catalytic roles of each elements and the rational design of Cr-free catalysts. The current study demonstrates, with temperature-programmed surface reaction (TPSR) spectroscopy (CO-TPSR, CO+H2O-TPSR, and HCOOH-TPSR), for the first time that the HT-WGS reaction follows the redox mechanism and that the associative mechanism does not take place." @default.
• W2331028144 created "2016-06-24" @default.
• W2331028144 creator A5052454489 @default.
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• W2331028144 date "2016-03-31" @default.
• W2331028144 modified "2023-10-18" @default.
• W2331028144 title "Resolving the Reaction Mechanism for H₂ Formation from High-Temperature Water–Gas Shift by Chromium–Iron Oxide Catalysts" @default.
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• W2331028144 doi "https://doi.org/10.1021/acscatal.6b00659" @default.
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