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- W2331308839 abstract "We report a systematic investigation of the electronic structure of chemisorbed alkali atoms (Li-Cs) on a Ag(111) surface by two-photon photoemission spectroscopy. Angle-resolved two-photon photoemission spectra are obtained for 0-0.1 monolayer coverage of alkali atoms. The interfacial electronic structure as a function of periodic properties and the coverage of alkali atoms is observed and interpreted assuming ionic adsorbate/substrate interaction. The energy of the alkali atom σ-resonance at the limit of zero coverage is primarily determined by the image charge interaction, whereas at finite alkali atom coverages, it follows the formation of a dipolar surface field. The coverage- and angle-dependent two-photon photoemission spectra provide information on the photoinduced charge-transfer excitation of adsorbates on metal surfaces. This work complements the previous work on alkali/Cu(111) chemisorption [Phys. Rev. B 2008, 78, 085419]." @default.
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- W2331308839 date "2011-04-20" @default.
- W2331308839 modified "2023-09-26" @default.
- W2331308839 title "Two-Photon Photoemission Study of the Coverage-Dependent Electronic Structure of Chemisorbed Alkali Atoms on a Ag(111) Surface" @default.
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- W2331308839 doi "https://doi.org/10.1021/jp111932r" @default.
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