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- W2331805265 endingPage "2888" @default.
- W2331805265 startingPage "2874" @default.
- W2331805265 abstract "Hydro/solvothermal and bilayered-diffusion methods using pyridine (py), 3-methylpyridine (3-mpy), and 4-methylpyridine (4-mpy) as weak bases and small terminal ligands generated seven CoII, MnII, and NiII two-dimensional (2D) coordination polymers with di-, trinuclear metal clusters as secondary building units (SBUs) from an organic bridging ligand, 1,1′-biphenyl-3,3′-dicarboxylic acid (H2L). Coordination polymers based on trinuclear SBUs are {[Co3(L)3(py)2](py)}n (1) and [Mn3(L)3(py)2(H2O)2]n (4), and those based on dinuclear SBUs are {[Co2(L)2(py)3(H2O)2](py)(CH3OH)}n (2), [Ni2(L)2(py)4(H2O)]n (3), {[Mn2(L)2(py)3(H2O)2](py)2(CH3CH2OH)}n (5), {[Mn2(L)2(3-mpy)4(H2O)](CH3OH)0.5}n (6), and [Mn2(L)2(4-mpy)2]n (7). Further structural analysis indicates that 1, 4, and 7 have a (4,4) grid layered structure and 2, 3, 5, and 6 possess a (3,6) sheet structure. Magnetization studies show the existence of ferromagnetic coupling for 1 with a positive zJ value of 0.97 cm–1, weak antiferromagnetic coupling for 2 (−E2/k = −4.6 K), very weak antiferromagnetic coupling for 3 with a small negative J value of −0.17 cm–1, weak or medium antiferromagnetic couplings for 4, 5, and 6 with the negative J values of −1.17, −1.53, and −1.62 cm–1, respectively, and very strong antiferromagnetic coupling for 7 with a very large negative J value of −16.62 cm–1." @default.
- W2331805265 created "2016-06-24" @default.
- W2331805265 creator A5025270767 @default.
- W2331805265 creator A5043238380 @default.
- W2331805265 creator A5058135877 @default.
- W2331805265 creator A5077420142 @default.
- W2331805265 date "2011-05-20" @default.
- W2331805265 modified "2023-10-12" @default.
- W2331805265 title "A Series of Two-Dimensional Co(II), Mn(II), and Ni(II) Coordination Polymers with Di- or Trinuclear Secondary Building Units Constructed by 1,1′-Biphenyl-3,3′-Dicarboxylic Acid: Synthesis, Structures, and Magnetic Properties" @default.
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