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• W2332861710 endingPage "6308" @default.
• W2332861710 startingPage "6302" @default.
• W2332861710 abstract "The ionic liquid 1-ethyl-3-methylimidazolium bis(trifluoromethylsulfonyl)imide ([emim][Tf2N]) offers new ways to modulate the electrochemical reduction of carbon dioxide. [emim][Tf2N], when present as the supporting electrolyte in acetonitrile, decreases the reduction overpotential at a Pb electrode by 0.18 V as compared to tetraethylammonium perchlorate as the supporting electrolyte. More interestingly, the ionic liquid shifts the reaction course during the electrochemical reduction of carbon dioxide by promoting the formation of carbon monoxide instead of oxalate anion. With increasing concentration of [emim][Tf2N], a carboxylate species with reduced CO2 covalently bonded to the imidazolium ring is formed along with carbon monoxide. The results highlight the catalytic effects of the medium in modulating the CO2 reduction products." @default.
• W2332861710 created "2016-06-24" @default.
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• W2332861710 creator A5061425161 @default.
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• W2332861710 date "2014-05-22" @default.
• W2332861710 modified "2023-10-16" @default.
• W2332861710 title "Switching the Reaction Course of Electrochemical CO₂ Reduction with Ionic Liquids" @default.
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• W2332861710 doi "https://doi.org/10.1021/la5009076" @default.
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• W2332861710 hasPublicationYear "2014" @default.
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