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- W2333612796 abstract "We studied the effect of initial substrate concentrations in the Belousov–Zhabotinsky (BZ) reaction on the optical transmittance self-oscillation behavior of a polymer chain consisting of N-isopropylacrylamide (NIPAAm) and a Fe catalyst ([Fe(bpy)3]). The driving force of this transmittance self-oscillation was the solubility difference between the reduced and oxidized states of the [Fe(bpy)3] moiety in the polymer chain. The amplitude of the soluble–insoluble self-oscillation of poly(NIPAAm-co-[Fe(bpy)3]) was significantly smaller than that of poly(NIPAAm-co-[Ru(bpy)3]). Theoretical simulation results attributed this behavior to the small difference in the solvent qualities, C*, of the reduced and oxidized states. Furthermore, we clarified that poly(NIPAAm-co-[Fe(bpy)3]) required a narrower concentration range of HNO3 to exhibit self-oscillation than poly(NIPAAm-co-[Ru(bpy)3]), since transmittance self-oscillation occurred only for [HNO3] = 0.3 M. The period of self-oscillation of poly(NIPAAm-co-[Fe(bpy)3]) in solution was controlled mainly by NaBrO3 concentration and was hardly influenced by the initial concentration of malonic acid." @default.
- W2333612796 created "2016-06-24" @default.
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- W2333612796 date "2014-06-06" @default.
- W2333612796 modified "2023-09-27" @default.
- W2333612796 title "Influence of Belousov–Zhabotinsky Substrate Concentrations on Autonomous Oscillation of Polymer Chains with Fe(bpy)<sub>3</sub> Catalyst" @default.
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- W2333612796 doi "https://doi.org/10.1021/jp500824e" @default.
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