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- W2333666240 abstract "The high Rydberg states probed by pulsed field ionization (PFI) zero–kinetic–energy (ZEKE) photoelectron spectroscopy are usually produced simultaneously with ions. These ions can have a profound influence on the appearance of a ZEKE photoelectron spectrum. It is now widely accepted that ions can lead to a considerable stabilization of high Rydberg states with respect to internal decay processes such as predissociation and autoionization. Two further effects of ions on the outcome of a ZEKE photoelectron spectroscopic experiment are demonstrated: (1) high ionic concentrations can modify the response of atomic and molecular Rydberg state populations to pulsed electric fields; (2) high ionic concentrations can have a detrimental effect on the resolution of a ZEKE photoelectron spectrum. These effects are illustrated by experimental results, which include the determination of the structure of a neutral molecule, the ammonium radical, by PFI–ZEKE spectroscopy." @default.
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- W2333666240 date "1997-08-15" @default.
- W2333666240 modified "2023-09-24" @default.
- W2333666240 title "On the role of ions in pulsed field ionization zero–kinetic–energy photoelectron spectroscopy" @default.
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- W2333666240 doi "https://doi.org/10.1098/rsta.1997.0076" @default.
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