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• W2334083133 abstract "A redox-reconfigurable catalyst derived from l-methionine and incorporating catalytic urea groups has been synthesized. This copper complex catalyzes the enantioselective addition of diethyl malonate to trans-β-nitrostyrene. Either enantiomer of the product can be predetermined by selection of the oxidation state of the copper ion. Enantiomeric excesses of up to 72% (S) and 70% (R) were obtained in acetonitrile. The ability of the catalyst to invert enantiomeric preference was reproduced with several different solvents and bases. Facile interconversion between the Cu2+ and Cu+ redox states allowed easy access to both active helical forms of the complex and, therefore, dial-in enantioselectivity." @default.
• W2334083133 created "2016-06-24" @default.
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• W2334083133 date "2012-05-07" @default.
• W2334083133 modified "2023-10-18" @default.
• W2334083133 title "A Redox-Reconfigurable, Ambidextrous Asymmetric Catalyst" @default.
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• W2334083133 doi "https://doi.org/10.1021/ja302283s" @default.
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