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• W2334128385 abstract "A nitrogen-rich ligand bis(1H-tetrazol-5-yl)amine (H(3)bta) was employed to isolate a new Fe(III) complex, Na(2)NH(4)[Fe(III)(Hbta)(3)]·3DMF·2H(2)O (1). Single crystal X-ray diffraction revealed that complex 1 consists of Fe(III) ions in an octahedral environment where each metal ion is coordinated by three Hbta(2-) ligands forming the [Fe(III)(Hbta)(3)](3-) core. Each unit is linked to two one-dimensional (1-D) Na(+)/solvent chains creating a two-dimensional (2-D) network. In addition, the presence of multiple hydrogen bonds in all directions between ammonium cation and ligands of different [Fe(III)(Hbta)(3)](3-) units generates a three-dimensional (3-D) network. Magnetic measurements confirmed that the Fe(III) center undergoes a Spin Crossover (SCO) at high temperature (T(1/2) = 460(10) K)." @default.
• W2334128385 created "2016-06-24" @default.
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• W2334128385 date "2013-02-06" @default.
• W2334128385 modified "2023-10-18" @default.
• W2334128385 title "High-Temperature Spin Crossover Behavior in a Nitrogen-Rich Fe^III-Based System" @default.
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• W2334128385 doi "https://doi.org/10.1021/ic301864d" @default.
• W2334128385 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/23387958" @default.
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