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- W2334303921 abstract "A Fourier transform spectrum of CH3Br between 4200 and 4600 cm−1, obtained on a BOMEM interferometer at a resolution of about 0.015 cm−1 is being analyzed, and several results have been obtained already for the CH379Br isotopomer. Here we give special emphasis to all those features which can lead to the identification and localization of the “unseen”v4+v5(A1,A2) system. Least squares calculations on assigned lines ofv2+v4±1(E) andv4±1+v5±1 (E) have been Performed allowing for thex−y Coriolis interaction of the former with all theE and (A1,A2) components ofv4+v5. Vibration-rotation constants have been estimated. The information on the unobserved (A1,A2) system ofv4+v5 is contained in the Coriolis perturbation of the δK=1 side ofv2+v4. The vibrational splitting of theA1 andA2 components ofv4+v5 is estimated to be small compared to the effect of theirz-axis Coriolis coupling. The least squares calculations give the origin of thev4+v5(A1,A2) system at 4477.65±4.04cm−1, but the examination of a localized perturbation on thepQ2 branch ofv4+v5(E), probably caused byl-resonance within thev4+v5 vibrational manifold, discloses the possibility of determining the above origin with better accuracy." @default.
- W2334303921 created "2016-06-24" @default.
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- W2334303921 date "1984-03-01" @default.
- W2334303921 modified "2023-09-26" @default.
- W2334303921 title "Evidence for theA 1 andA 2 components ofv 4+v 5 the infrared spectrum of methyl bromide" @default.
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- W2334303921 doi "https://doi.org/10.1007/bf03155927" @default.
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