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- W2334310064 abstract "Abstract Previous studies have suggested that the reaction of O 2 ( 1 Σ g + ) + N 2 O → NO + NO 2 may be a significant source of NO x in the atmosphere if the branching ratio of this channel is greater than ~1%. We have measured the overall rate coefficient (k 1 ) for the reaction of O 2 ( 1 Σ g + ) with N 2 O to be k 1 (295 K) = (1.06±0.14)×10 −13 cm 3 molecule −1 s −1 at 295 K and k 1 (T) = (7.48±1.66)×10 −14 exp[(87±40)/T] cm 3 molecule −1 s −1 as a function of temperature over the range 210–370 K. The yields of NO, NO 2 or O 3 that are possible reaction products from the title reaction were undetectably small. Also, the net loss of N 2 O from the title reaction was negligibly small. We report upper limits for the yields for the production of NO x , the production of O 3 and the loss of N 2 O (all at 298 K) to be < 2×10 −4 , < 1×10 −3 , and < 3×10 −3 , respectively. We conclude that the reaction of O 2 ( 1 Σ g + ) + N 2 O is neither a significant source of NO x in the atmosphere nor a significant sink for N 2 O." @default.
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- W2334310064 date "2010-08-01" @default.
- W2334310064 modified "2023-09-26" @default.
- W2334310064 title "Kinetics and Products of the Reaction O<sub>2</sub>(<sup>1</sup>Σ<sub>g</sub> <sup>+</sup>) with N<sub>2</sub>O" @default.
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- W2334310064 doi "https://doi.org/10.1524/zpch.2010.6137" @default.
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