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• W2334691022 startingPage "18222" @default.
• W2334691022 abstract "Electronic energy relaxation of Au144(SR)60q ligand-protected nanoclusters, where SR = SC6H13 and q = −1, 0, +1, and +2, was examined using femtosecond time-resolved transient absorption spectroscopy. The observed differential transient spectra contained three distinct components: (1) transient bleaches at 525 and 600 nm, (2) broad visible excited-state absorption (ESA), and (3) stimulated emission (SE) at 670 nm. The bleach recovery kinetics depended upon the excitation pulse energy and were thus attributed to electron–phonon coupling typical of metallic nanostructures. The prominent bleach at 525 nm was assigned to a core-localized plasmon resonance (CLPR). ESA decay kinetics were oxidation-state dependent and could be described using a metal-sphere charging model. The dynamics, emission energy, and intensity of the SE peak exhibited dielectric-dependent responses indicative of Superatom charge transfer states. On the basis of these data, the Au144(SR)60 system is the smallest-known nanocluster to exhibit quantifiable electron dynamics and optical properties characteristic of metals." @default.
• W2334691022 created "2016-06-24" @default.
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• W2334691022 date "2013-11-20" @default.
• W2334691022 modified "2023-10-03" @default.
• W2334691022 title "Optical Properties and Electronic Energy Relaxation of Metallic Au₁₄₄(SR)₆₀ Nanoclusters" @default.
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• W2334691022 doi "https://doi.org/10.1021/ja409998j" @default.
• W2334691022 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/24195472" @default.
• W2334691022 hasPublicationYear "2013" @default.
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