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• W2334756819 endingPage "4307" @default.
• W2334756819 startingPage "4304" @default.
• W2334756819 abstract "Intramolecular isomerization in pentacoordinate compounds can play an essential role for the adjustment of defined stereochemical information. Here, we present a conclusive mechanism of a stereocontrolled reaction on chiral dimethoxysilanes that opens new aspects in understanding the origin of creating silicon-centered chirality during a nucleophilic substitution process. By combining experimental, structural, and quantum chemical methods, we were able to disclose an interconversion process, based on consecutive Berry-type motions, as the most plausible mechanism for describing the stereochemical outcome in suchlike substitution reactions." @default.
• W2334756819 created "2016-06-24" @default.
• W2334756819 creator A5033600382 @default.
• W2334756819 creator A5073048622 @default.
• W2334756819 date "2015-03-30" @default.
• W2334756819 modified "2023-10-14" @default.
• W2334756819 title "Stereocontrol in Nucleophilic Substitution Reactions at Silicon: The Role of Permutation in Generating Silicon-Centered Chirality" @default.
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• W2334756819 doi "https://doi.org/10.1021/jacs.5b00861" @default.
• W2334756819 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/25803673" @default.
• W2334756819 hasPublicationYear "2015" @default.
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