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- W2334794051 abstract "A four-step synthesis of the antimalarial terpene cardamom peroxide, a 1,2-dioxepane-containing natural product, is reported from (-)-myrtenal and molecular oxygen. This highly concise route was guided by biosynthetic logic and enabled by an unusual manganese-catalyzed, tandem hydroperoxidation reaction. The absolute configuration of the cardamom peroxide is reported, and its mode of fragmentation following Fe(II)-mediated endoperoxide reduction is established. These studies reveal the generation of reactive intermediates distinct from previously studied endoperoxide natural products." @default.
- W2334794051 created "2016-06-24" @default.
- W2334794051 creator A5014800022 @default.
- W2334794051 creator A5057467468 @default.
- W2334794051 date "2014-03-27" @default.
- W2334794051 modified "2023-10-16" @default.
- W2334794051 title "Four-Step Synthesis of the Antimalarial Cardamom Peroxide via an Oxygen Stitching Strategy" @default.
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- W2334794051 doi "https://doi.org/10.1021/ja502208z" @default.
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