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• W2334953073 startingPage "15905" @default.
• W2334953073 abstract "Uranium and uranium dioxide carbonyl cations produced by laser vaporization are studied with mass-selected ion infrared spectroscopy in the C-O stretching region. Dissociation patterns, spectra, and quantum chemical calculations establish that the fully coordinated ions are U(CO)(8)(+) and UO(2)(CO)(5)(+), with D(4d) square antiprism and D(5h) pentagonal bipyramid structures. Back-bonding in U(CO)(8)(+) causes a red-shifted CO stretch, but back-donation is inefficient for UO(2)(CO)(5)(+), producing a blue-shifted CO stretch characteristic of nonclassical carbonyls." @default.
• W2334953073 created "2016-06-24" @default.
• W2334953073 creator A5024641277 @default.
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• W2334953073 creator A5062631568 @default.
• W2334953073 date "2010-11-17" @default.
• W2334953073 modified "2023-10-16" @default.
• W2334953073 title "Infrared spectroscopy of extreme coordination: the carbonyls of U(+) and UO(2)(+)." @default.
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• W2334953073 doi "https://doi.org/10.1021/ja1077365" @default.
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• W2334953073 hasPublicationYear "2010" @default.
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