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• W2334966072 endingPage "195602" @default.
• W2334966072 startingPage "195602" @default.
• W2334966072 abstract "The ability to easily manufacture nanostructures with a desirable attribute, such as well-defined size and shape, especially from any given initial shapes or sizes of the material, will be helpful towards accelerating the use of nanomaterials in various applications. In this work we report the transformation of discontinuous irregular nanostructures (DIN) of silver metal by rapid heating under a bulk fluid layer. Ag films were changed into DIN by dewetting in air and subsequently heated by nanosecond laser pulses under water. Our findings show that the DIN first ripens into elongated structures and then breaks up into nanoparticles. From the dependence of this behavior on laser fluence we found that under water irradiation reduced the rate of ripening and also decreased the characteristic break-up length scale of the elongated structures. This latter result was qualitatively interpreted as arising from a Rayleigh-Plateau instability modified to yield significantly smaller length scales than the classical process due to pressure gradients arising from the rapid evaporation of water during laser melting. These results demonstrate that it is possible to fabricate a dense collection of monomodally sized Ag nanoparticles with significantly enhanced plasmonic quality starting from the irregular shaped materials. This can be beneficial towards transforming discontinuous Ag films into nanostructures with useful plasmonic properties, that are relevant for biosensing applications." @default.
• W2334966072 created "2016-06-24" @default.
• W2334966072 creator A5057818638 @default.
• W2334966072 creator A5075410026 @default.
• W2334966072 creator A5084747382 @default.
• W2334966072 date "2016-04-04" @default.
• W2334966072 modified "2023-09-24" @default.
• W2334966072 title "Transformation of irregular shaped silver nanostructures into nanoparticles by under water pulsed laser melting" @default.
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• W2334966072 doi "https://doi.org/10.1088/0957-4484/27/19/195602" @default.
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• W2334966072 hasPublicationYear "2016" @default.
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