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- W2334998439 abstract "The catalytic performance of Al2O3-supported monometallic and bimetallic catalysts in selective hydrogenation of 1,3-butadiene in the presence of 1-butene under liquid phase conditions was studied. Bimetallic catalysts were prepared by the coimpregnation method with the required amounts of the precursors salts [Ni(NO3)2·6H2O and Pd(NH3)4Cl2·H2O] over pellet-form γ-Al2O3 with a constant content of Pd (0.5 wt%) and varying Ni/Pd atomic ratio (0.25, 0.5, 0.75, and 1) obtaining egg-shell profiles of the active components. The catalysts were characterized by X-ray diffraction, temperature-programmed techniques, such as reduction in hydrogen and desorption of ammonia, N2 physisorption, and transmission electron microscopy. The catalytic test showed that the 1,3-butadiene was selectively hydrogenated when bimetallic catalysts were used. The addition of Ni to the Pd-based catalysts suppressed n-butane formation and increased recovery of 1-butene at medium conversion. Therefore, it was observed an improved catalytic performance of the bimetallic catalysts being highest in the case of the 1NiPd/Al2O3." @default.
- W2334998439 created "2016-06-24" @default.
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- W2334998439 date "2016-04-02" @default.
- W2334998439 modified "2023-10-15" @default.
- W2334998439 title "Selective hydrogenation of 1,3-butadiene in presence of 1-butene under liquid phase conditions with NiPd/Al2O3 catalysts" @default.
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- W2334998439 doi "https://doi.org/10.1007/s13203-016-0149-y" @default.
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